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Kätchen K. Lachmayr Prof. Lawrence R. Sita 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(9):3591-3595
Incorporation of small amounts of α-tocopherol (vitamin E) in blends with the cellobiose–triazole-linked atactic poly(4-methyl-1-pentene) (CB-aPMP) sugar–polyolefin conjugate can be used to exert external control over thermotropic phase behavior and provide access to non-canonical soft matter Frank–Kasper A15 and σ phases. These results establish a paradigm that can be used for the further design and development of scalable quantities of soft matter FK phases of increased structural complexity and functional capability. 相似文献
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Joachim Toft 《Applied and Computational Harmonic Analysis》2019,46(1):154-176
We extend Feichtinger's minimality property on the smallest non-trivial time-frequency shift invariant Banach space, to the quasi-Banach case. Analogous properties are deduced for certain matrix spaces.We use these results to prove that the pseudo-differential operator is a Schatten-q operator from to and r-nuclear operator from to when for suitable p, q and r in . 相似文献
4.
The enhancement of teleportation fidelity by weak measurement or quantum measurement reversal is investigated. One qubit of a maximally entangled state undergoes the amplitude damping, and the subsequent application of weak measurement or quantum measurement reversal could improve the teleportation fidelity beyond the classical region. The improvement could not be attributed to the increasing of entanglement, quantum discord, classical correlation or total correlation. We declare that it should be owed to the probabilistic nature of the method. 相似文献
5.
Dr. Yutao Liu Hui Chen Tong Li Yongheng Ren Hui Wang Zhengxuan Song Jianhui Li Prof. Qiang Zhao Prof. Jinping Li Prof. Libo Li 《Angewandte Chemie (International ed. in English)》2023,62(37):e202309095
Polycrystalline metal–organic framework (MOF) layers hold great promise as molecular sieve membranes for efficient gas separation. Nevertheless, the high crystallinity tends to cause inter-crystalline defects/cracks in the nearby crystals, which makes crystalline porous materials face a great challenge in the fabrication of defect-free membranes. Herein, for the first time, we demonstrate the balance between crystallinity and film formation of MOF membrane through a facile in situ modulation strategy. Monocarboxylic acid was introduced as a modulator to regulate the crystallinity via competitive complexation and thus concomitantly control the film-forming state during membrane growth. Through adjusting the ratio of modulator acid/linker acid, an appropriate balance between this structural “trade-off” was achieved. The resulting MOF membrane with moderate crystallinity and coherent morphology exhibits molecular sieving for H2/CO2 separation with selectivity up to 82.5. 相似文献
6.
In this Note we study the effects of the temperature modulation, applied at the horizontal boundaries, on the onset of convection of a horizontal liquid Maxwellian layer. It is assumed that the temperature imposed features a steady component and a time dependent component. To analyse the effect of the temperature modulation, the study is restricted to a linear stability analysis. Thus the Floquet theory and a technique of converting a boundary value problem to an initial value problem are used to solve the system of equations corresponding to the onset of convection. Results obtained may be used to characterize the influence of modulation effects and that of the viscoelastic nature of liquid on the critical Rayleigh number. To cite this article: B. Oukada et al., C. R. Mecanique 334 (2006). 相似文献
7.
We consider the problem of laminar mixed convection flow between parallel, vertical and uniformly heated plates where the governing dimensionless parameters are the Prandtl, Rayleigh and Reynolds numbers. Using the method based on the centre manifold theorem which was derived from the general theory of dynamical systems, we reduce a three-dimensional simplified model of ordinary differential amplitude equations emanating from the original Navier-Stokes system of the problem in the vicinity of a trivial stationary solution. We have found that when the forcing parameter, the Rayleigh number, increases beyond the critical value Ras, the stationary solution is a pitchfork bifurcation point of the system. 相似文献
8.
本文研究了一端弹性支撑的并列双柱和串列双圆柱在气流中自由端的振幅响应,与单圆柱相比,在小间距时,串列双圆柱中前柱的横向振幅受到较强的激励。而在大间距时,振幅受到抑制,特别当L/D=3.5和4.0时,其振幅响应仅为单柱的1/3左右,而对于后柱,则在大间距时,纵向振幅响应有所增大,而且后柱的振幅响应要比前柱的大得多,而并列双圆柱的自由端振幅基本上受到抑制,在T/D>3.0之后,干扰很快减小到接近单个圆 相似文献
9.
Here, the large amplitude free flexural vibration behaviors of thin laminated composite skew plates are investigated using finite element approach. The formulation includes the effects of shear deformation, in-plane and rotary inertia. The geometric non-linearity based on von Karman's assumptions is introduced. The non-linear governing equations obtained employing Lagrange's equations of motion are solved using the direct iteration technique. The variation of non-linear frequency ratios with amplitudes is brought out considering different parameters such as skew angle, number of layers, fiber orientation, boundary condition and aspect ratio. The influence of higher vibration modes on the non-linear dynamic behavior of laminated skew plates is also highlighted. The present study reveals the redistribution of vibrating mode shape at certain amplitude of vibration depending on geometric and lamination parameters of the plate. Also, the degree of hardening behavior increases with the skew angle and its rate of change depends on the level of amplitude of vibration. 相似文献
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